Document Detail


The ybxI gene of Bacillus subtilis 168 encodes a class D beta-lactamase of low activity.
MedLine Citation:
PMID:  14742199     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The ybxI gene of Bacillus subtilis 168 encodes a preprotein of 267 amino acid residues, including a putative signal peptide of 23 residues. The YbxI primary structure exhibits high similarity scores with two members of the superfamily of the serine penicillin-recognizing enzymes: the class D beta-lactamases and the hydrophilic carboxy-terminal domains of the BlaR and MecR penicillin receptors. To determine the function and the activity of this putative penicillin-recognizing enzyme, we have subcloned the ybxI gene in the pET-26b expression vector. Transformation of Escherichia coli BL21(DE3) by the recombinant plasmid pCIP51 resulted in the export of the mature YbxI in the periplasm as a water-soluble protein. The recombinant protein was purified to 95% homogeneity. YbxI interacts with several beta-lactam antibiotics and can hydrolyze some of them. YbxI is not inactivated by clavulanic acid. The YbxI function and its enzymatic activity in B. subtilis remain unknown. The acyl-enzyme obtained after incubation of YbxI with a fluorescent derivative of ampicillin can be detected by sodium dodecyl sulfate-polyacrylamide gel electrophoresis, confirming that YbxI can be acylated by beta-lactam antibiotics. YbxI does not hydrolyze some of the standard substrates of D-alanyl-D-alanine peptidases, the targets of penicillin. YbxI belongs to the penicillin-recognizing enzyme family but has an activity intermediate between those of a penicillin-binding protein and a beta-lactamase.
Authors:
Maria-Luigi Colombo; Sophie Hanique; Stéphane L Baurin; Cédric Bauvois; Kris De Vriendt; Jozef J Van Beeumen; Jean-Marie Frère; Bernard Joris
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  Antimicrobial agents and chemotherapy     Volume:  48     ISSN:  0066-4804     ISO Abbreviation:  Antimicrob. Agents Chemother.     Publication Date:  2004 Feb 
Date Detail:
Created Date:  2004-01-26     Completed Date:  2004-03-11     Revised Date:  2013-04-18    
Medline Journal Info:
Nlm Unique ID:  0315061     Medline TA:  Antimicrob Agents Chemother     Country:  United States    
Other Details:
Languages:  eng     Pagination:  484-90     Citation Subset:  IM    
Affiliation:
Centre d'Ingénierie des Protéines, Institut de Chimie B6a, Université de Liège, Sart Tilman, B-4000 Liège 1, Belgium.
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MeSH Terms
Descriptor/Qualifier:
Amino Acid Sequence
Bacillus subtilis / drug effects,  enzymology*,  genetics*
Bacterial Proteins
Bicarbonates / pharmacology
Carrier Proteins
Cephalosporins / metabolism
Electrophoresis, Polyacrylamide Gel
Genes, Bacterial / genetics*
Hexosyltransferases
Hydrolysis
Kinetics
Molecular Sequence Data
Muramoylpentapeptide Carboxypeptidase
Penicillin-Binding Proteins
Peptidoglycan / metabolism
Peptidyl Transferases
Plasmids / genetics
RNA, Bacterial / biosynthesis
RNA, Messenger / biosynthesis
Reverse Transcriptase Polymerase Chain Reaction
beta-Lactamases / biosynthesis*,  genetics*
Chemical
Reg. No./Substance:
0/Bacterial Proteins; 0/Bicarbonates; 0/Carrier Proteins; 0/Cephalosporins; 0/Penicillin-Binding Proteins; 0/Peptidoglycan; 0/RNA, Bacterial; 0/RNA, Messenger; EC 2.3.2.12/Peptidyl Transferases; EC 2.4.1.-/Hexosyltransferases; EC 3.4.17.8/Muramoylpentapeptide Carboxypeptidase; EC 3.5.2.6/beta-Lactamases; EWP54G0J8F/nitrocefin
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