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On the choice of heteronuclear dipolar decoupling scheme in solid-state NMR.
MedLine Citation:
PMID:  20870436     Owner:  NLM     Status:  In-Process    
Abstract/OtherAbstract:
We present here a comparison of different heteronuclear dipolar decoupling sequences at the moderate magic-angle spinning (MAS) frequency (ν(r)) of 30 kHz. The radio-frequency (RF) amplitude (ν₁) ranges from the low power (ν₁<ν(r)) to the high power regime (ν₁>2ν(r)) and includes the rotary resonance conditions (ν₁=nν(r)) where n=1, 2. For decoupling at the rotary resonance condition, we recently introduced a modification of TPPM, namely high-phase TPPM, whose properties will be discussed here. Finally, based on earlier published and current experimental results we suggest the optimal sequence for heteronuclear dipolar decoupling at any RF amplitude and MAS frequencies up to 35 kHz.
Authors:
Subhradip Paul; N D Kurur; P K Madhu
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Publication Detail:
Type:  Journal Article     Date:  2010-09-09
Journal Detail:
Title:  Journal of magnetic resonance (San Diego, Calif. : 1997)     Volume:  207     ISSN:  1096-0856     ISO Abbreviation:  J. Magn. Reson.     Publication Date:  2010 Nov 
Date Detail:
Created Date:  2010-10-18     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9707935     Medline TA:  J Magn Reson     Country:  United States    
Other Details:
Languages:  eng     Pagination:  140-8     Citation Subset:  IM    
Copyright Information:
Copyright © 2010 Elsevier Inc. All rights reserved.
Affiliation:
Department of Chemical Sciences, Tata Institute of Fundamental Research, Homi Bhabha Road, Colaba, Mumbai 400 005, India.
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