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Wewakamide A and Guineamide G, Cyclic Depsipeptides from the Marine Cyanobacteria Lyngbya semiplena and Lyngbya majuscula.
MedLine Citation:
PMID:  21952369     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
Two new cyclic depsipeptides wewakamide A (1) and guineamide G (2) have been isolated from the marine cyanobacterium Lyngbya semiplena and Lyngbya majuscula, respectively, collected from Papua New Guinea. The amino and hydroxy acid partial structures of wewakamide A and guineamide G were elucidated through extensive spectroscopic techniques, including HR-FABMS, 1D 1H and 13C NMR, as well as 2D COSY, HSQC, HSQCTOCSY, and HMBC spectra. The sequence of the residues of wewakamide A was determined through a combination of ESI-MS/MS, HMBC, and ROESY. Wewakamide A possesses a beta-amino acid, 3-amino-2-methylbutanoic acid (Maba) residue, which has only been previously identified in two natural products, guineamide B (3) and dolastatin D (4). Although both new compounds (1,2) showed potent brine shrimp toxicity, only guineamide G displayed significant cytotoxicity to a mouse neuroblastoma cell line with LC50 values of 2.7 micrometer.
Authors:
Bingnan Han; Harald Gross; Kerry L McPhail; Doug Goeger; Claudia S Maier; William H Gerwick
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Publication Detail:
Type:  -    
Journal Detail:
Title:  Journal of microbiology and biotechnology     Volume:  21     ISSN:  1738-8872     ISO Abbreviation:  -     Publication Date:  2011 Sep 
Date Detail:
Created Date:  2011-9-28     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9431852     Medline TA:  J Microbiol Biotechnol     Country:  -    
Other Details:
Languages:  ENG     Pagination:  930-936     Citation Subset:  -    
Affiliation:
Department of Ocean Science and Engineering, Zhejiang University, Hangzhou, China 310028.
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