Document Detail


Ultrasound artificially nucleated bubbles and their sonochemical radical production.
MedLine Citation:
PMID:  22939003     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
We describe the ejection of bubbles from air-filled pits micromachined on a silicon surface when exposed to ultrasound at a frequency of approximately 200kHz. As the pressure amplitude is increased the bubbles ejected from the micropits tend to be larger and they interact in complex ways. With more than one pit, there is a threshold pressure beyond which the bubbles follow a trajectory parallel to the substrate surface and converge at the center point of the pit array. We have determined the size distribution of bubbles ejected from one, two and three pits, for three different pressure amplitudes and correlated them with sonochemical OH() radical production. Experimental evidence of shock wave emission from the bubble clusters, deformed bubble shapes and jetting events that might lead to surface erosion are presented. We describe numerical simulations of sonochemical conversion using the empirical bubble size distributions, and compare the calculated values with experimental results.
Authors:
David Fernandez Rivas; Laura Stricker; Aaldert G Zijlstra; Han J G E Gardeniers; Detlef Lohse; Andrea Prosperetti
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Publication Detail:
Type:  JOURNAL ARTICLE     Date:  2012-8-9
Journal Detail:
Title:  Ultrasonics sonochemistry     Volume:  -     ISSN:  1873-2828     ISO Abbreviation:  Ultrason Sonochem     Publication Date:  2012 Aug 
Date Detail:
Created Date:  2012-9-3     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9433356     Medline TA:  Ultrason Sonochem     Country:  -    
Other Details:
Languages:  ENG     Pagination:  -     Citation Subset:  -    
Copyright Information:
Copyright © 2012 Elsevier B.V. All rights reserved.
Affiliation:
Mesoscale Chemical Systems Group, MESA+ Research Institute, University of Twente, P.O. Box 217, 7500 AE Enschede, The Netherlands.
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