Document Detail


Ultra-trace determination of S-nitrosothiols in blood samples by spectrofluorimetry with 8-(3',4'-diaminophenyl)-difluoroboradiaza-s-indacene.
MedLine Citation:
PMID:  17531528     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Increasing evidence suggests that S-nitrosothiols (RSNO) may represent naturally occurring nitric oxide (NO) surrogates and function as intermediates in NO metabolism. In this work, a simple, sensitive, and selective micromethod is developed and validated for quantification of RSNO. A fluorescent probe 8-(3',4'-diaminophenyl)-difluoroboradiaza-s-indacence (DABODIPY) is firstly used to label RSNO. The derivatization reaction is performed in aqueous medium at 30 degrees C for 15min in the presence of 6x10(-5)molL(-1)Hg2+ and the derivative is detected by fluorescence at lambda(ex)/lambda(em)=500/510nm. A linear function of concentration in the range of (2.0-600.0)x10(-8)molL(-1) is observed with a correlation coefficient of 0.9992 and detection limit of 1.2x10(-9)molL(-1) (S/N=3). This technique has been successfully applied to quantify RSNO in some human blood samples including healthy persons and patients suffering from cardiovascular diseases.
Authors:
Ke-Jing Huang; Chun-Xuan Xu; Wan-Zhen Xie; Hua-Shan Zhang; Hong Wang
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't     Date:  2007-04-24
Journal Detail:
Title:  Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy     Volume:  69     ISSN:  1386-1425     ISO Abbreviation:  Spectrochim Acta A Mol Biomol Spectrosc     Publication Date:  2008 Feb 
Date Detail:
Created Date:  2008-02-04     Completed Date:  2008-05-22     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9602533     Medline TA:  Spectrochim Acta A Mol Biomol Spectrosc     Country:  England    
Other Details:
Languages:  eng     Pagination:  437-42     Citation Subset:  IM    
Affiliation:
Department of Chemistry, Wuhan University, Wuhan 430072, PR China.
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MeSH Terms
Descriptor/Qualifier:
Boron Compounds* / chemistry
Glutathione / analogs & derivatives,  chemistry
Heterocyclic Compounds, 3-Ring* / chemistry
Humans
Ions / chemistry
Molecular Structure
Nitro Compounds / chemistry
S-Nitrosothiols / blood*,  chemistry
Spectrometry, Fluorescence / methods*
Chemical
Reg. No./Substance:
0/8-(3',4'-diaminophenyl)-difluoroboradiaza-S-indacence; 0/Boron Compounds; 0/Heterocyclic Compounds, 3-Ring; 0/Ions; 0/Nitro Compounds; 0/S-Nitrosothiols; 0/S-nitroglutathione; 70-18-8/Glutathione

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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