Document Detail

Two-photon excited fluorescence and molecular reorientations in liquid solutions.
MedLine Citation:
PMID:  17578656     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Theoretical expressions are derived that relate the two-photon excited fluorescence depolarisation experiments to the molecular symmetry and the rotational motions of fluorescent molecules. Diffusive rotational motions in liquid solvents are considered, as well as the influence of fast unresolved motions (e.g. librations). The results obtained are compared with one-photon excited fluorescence depolarisation experiments. The derived theoretical expressions can be applied for detailed analyses of the molecular rotation in solvent. Several of the results are useful for determining and assigning the components of two-photon absorption tensors.
Linus Ryderfors; Emad Mukhtar; Lennart B-A Johansson
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Publication Detail:
Type:  Journal Article     Date:  2007-06-21
Journal Detail:
Title:  Journal of fluorescence     Volume:  17     ISSN:  1053-0509     ISO Abbreviation:  J Fluoresc     Publication Date:  2007 Sep 
Date Detail:
Created Date:  2007-08-21     Completed Date:  2007-11-07     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9201341     Medline TA:  J Fluoresc     Country:  United States    
Other Details:
Languages:  eng     Pagination:  466-80     Citation Subset:  -    
Department of Photochemistry and Molecular Science, Uppsala University, 751 20-Uppsala, Sweden.
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