Document Detail


Synthesis, structural characterization, thermal and electrochemical studies of mixed ligand Cu(II) complexes containing 2-phenyl-3-(benzylamino)-1,2-dihydroquinazoline-4-(3H)-one and bidentate N-donor ligands.
MedLine Citation:
PMID:  19828363     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Some mixed ligand Cu(II) complexes of the type [Cu(L)(en)X(2)] (1a-3a), [Cu(L)(en)](ClO(4))(2) (4a), [Cu(L)(phen)X(2)] (1b-3b) and [Cu(L)(phen)](ClO(4))(2) (4b) [where L = 2-phenyl-3-(benzylamino)-1,2-dihydroquinazoline-4-(3H)-one; en = ethylenediamine; phen = 1,10-phenanthroline; X = Cl(-), N(3)(-) and NCS(-)] have been prepared. The complexes were characterized on the basis of elemental analysis, molar conductance, magnetic moment, IR, UV-vis, mass, ESR and thermal studies. On the basis of electronic spectral data and magnetic susceptibility measurement octahedral geometry has been proposed for 1a-3a and 1b-3b and square-planer geometry for 4a and 4b. The ESR spectral data of complexes provided information about their structure on the basis of Hamiltonian parameters and degree of covalency. The electrochemical behaviour of mixed ligand Cu(II) complexes was studied which showed that complexes of phen appear at more positive potential as compared to those for corresponding en complexes.
Authors:
V A Sawant; B A Yamgar; S K Sawant; S S Chavan
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Publication Detail:
Type:  Journal Article     Date:  2009-09-19
Journal Detail:
Title:  Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy     Volume:  74     ISSN:  1873-3557     ISO Abbreviation:  Spectrochim Acta A Mol Biomol Spectrosc     Publication Date:  2009 Dec 
Date Detail:
Created Date:  2009-11-10     Completed Date:  2010-01-29     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9602533     Medline TA:  Spectrochim Acta A Mol Biomol Spectrosc     Country:  England    
Other Details:
Languages:  eng     Pagination:  1100-6     Citation Subset:  IM    
Affiliation:
Department of Chemistry, Shivaji University, Kolhapur (MS) 416 004, India.
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MeSH Terms
Descriptor/Qualifier:
Copper / chemistry*
Differential Thermal Analysis
Electrochemistry*
Electron Spin Resonance Spectroscopy
Electrons
Ligands
Magnetics
Quinazolines / chemistry*
Spectrophotometry, Infrared
Temperature*
Thermogravimetry
Chemical
Reg. No./Substance:
0/2-phenyl-3-(benzylamino)-1,2-dihydroquinazoline-4-(3H)-one; 0/Ligands; 0/Quinazolines; 7440-50-8/Copper

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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