Document Detail


Synthesis, analytical characterization and use of octakis(2,3-di-O-methyl-6-O-sulfo)-gamma-cyclodextrin, a novel, single-isomer, chiral resolving agent in low-pH background electrolytes.
MedLine Citation:
PMID:  12569527     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The third member of the family of single-isomer, sulfated gamma-cyclodextrins, the sodium salt of octakis(2,3-di-O-methyl-6-O-sulfo)-gamma-cyclodextrin has been synthesized, analytically characterized and used for the capillary electrophoretic separation of the enantiomers of nonionic, weak acid and weak base analytes in low-pH aqueous background electrolytes. Though octakis(2,3-di-O-methyl-6-O-sulfo)-gamma-cyclodextrin complexes less strongly with many of the analytes tested than the other members of the single-isomer, 6-O-sulfo gamma-cyclodextrin family, such as octa(6-O-sulfo)-gamma-cyclodextrin and octakis(2,3-di-O-acetyl-6-O-sulfo)-gamma-cyclodextrin, it offers excellent separation selectivities, often complementary to those of both the single-isomer, 6-O-sulfo beta-cyclodextrins and 6-O-sulfo gamma-cyclodextrins. Rapid, efficient enantiomer separations were observed for a large number of structurally diverse analytes in acidic aqueous background electrolytes.
Authors:
M Brent Busby; Peniel Lim; Gyula Vigh
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  Electrophoresis     Volume:  24     ISSN:  0173-0835     ISO Abbreviation:  Electrophoresis     Publication Date:  2003 Jan 
Date Detail:
Created Date:  2003-02-05     Completed Date:  2003-12-04     Revised Date:  2006-11-15    
Medline Journal Info:
Nlm Unique ID:  8204476     Medline TA:  Electrophoresis     Country:  Germany    
Other Details:
Languages:  eng     Pagination:  351-62     Citation Subset:  IM    
Affiliation:
Department of Chemistry, Texas A & M University, College Station, TX 77842, USA.
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MeSH Terms
Descriptor/Qualifier:
Cyclodextrins / chemical synthesis*,  chemistry
Electrolytes
Electrophoresis, Capillary / methods*
Hydrogen-Ion Concentration
Indicators and Reagents
Organic Chemicals / isolation & purification
Stereoisomerism
gamma-Cyclodextrins*
Chemical
Reg. No./Substance:
0/Cyclodextrins; 0/Electrolytes; 0/Indicators and Reagents; 0/Organic Chemicals; 0/gamma-Cyclodextrins; 0/octakis(2,3-dimethyl-6-O-sulfo)-gamma-cyclodextrin

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