Document Detail


Synthesis and structural aspects of N-triflylphosphoramides and their calcium salts--highly acidic and effective Brønsted acids.
MedLine Citation:
PMID:  20922721     Owner:  NLM     Status:  In-Process    
Abstract/OtherAbstract:
Recently, 1,1'-bi-2-naphthol (BINOL)-based N-triflylphosphoramides emerged as a new class of potent Brønsted acid catalysts. In this paper we describe the efficient synthesis of various BINOL-based N-triflylphosphoramides and their calcium salts. Furthermore, X-ray crystal structure analysis combined with energy-dispersive X-ray spectroscopy (EDX) measurements confirmed that the synthesised chiral N-triflylphosphoramides are highly acidic metal-free catalysts.
Authors:
Magnus Rueping; Boris J Nachtsheim; René M Koenigs; Winai Ieawsuwan
Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Chemistry (Weinheim an der Bergstrasse, Germany)     Volume:  16     ISSN:  1521-3765     ISO Abbreviation:  Chemistry     Publication Date:  2010 Nov 
Date Detail:
Created Date:  2010-11-16     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9513783     Medline TA:  Chemistry     Country:  Germany    
Other Details:
Languages:  eng     Pagination:  13116-26     Citation Subset:  -    
Affiliation:
RWTH Aachen University, Institute of Organic Chemistry, Landoltweg 1, 52074 Aachen, Germany. magnus.rueping@rwth-aachen.de
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