Document Detail


Surface and blood-contacting properties of alkylsiloxane monolayers supported on silicone rubber.
MedLine Citation:
PMID:  7622539     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Self-assembled monolayers of alkylsiloxanes supported on polydimethyl siloxane (PDMS) rubber were used as model systems to study the relation between blood compatibility and surface chemistry. The inner lumen of PDMS tubes was first treated with an oxygen plasma. The resultant oxidized surfaces were postderivatized by reacting them with alkyltrichlorosilanes to form the monolayer films. The chemical properties of the monolayers were controlled by varying the head-group chemical compositions. Surface derivatization was verified using variable-angle X-ray photoelectron spectroscopy (XPS or ESCA). Blood compatibility was evaluated using a canine ex vivo arteriovenous series shunt model. Surfaces grafted with hydrophobic head-groups as -CH3 and -CF3 had significantly lower platelet and fibrinogen deposition than the surfaces composed of hydrophilic groups such as -CO2CH3, -(CH2CH2O)3COCH3, and -(OCH2CH2)3OH.
Authors:
J H Silver; R W Hergenrother; J C Lin; F Lim; H B Lin; T Okada; M K Chaudhury; S L Cooper
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't; Research Support, U.S. Gov't, P.H.S.    
Journal Detail:
Title:  Journal of biomedical materials research     Volume:  29     ISSN:  0021-9304     ISO Abbreviation:  J. Biomed. Mater. Res.     Publication Date:  1995 Apr 
Date Detail:
Created Date:  1995-08-31     Completed Date:  1995-08-31     Revised Date:  2007-11-14    
Medline Journal Info:
Nlm Unique ID:  0112726     Medline TA:  J Biomed Mater Res     Country:  UNITED STATES    
Other Details:
Languages:  eng     Pagination:  535-48     Citation Subset:  IM    
Affiliation:
Department of Chemical Engineering, University of Wisconsin, Madison 53706, USA.
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MeSH Terms
Descriptor/Qualifier:
Animals
Biocompatible Materials*
Blood*
Blood Coagulation
Dimethylpolysiloxanes*
Dogs
Electron Probe Microanalysis
Fibrinogen / metabolism
Platelet Adhesiveness
Silanes*
Silicones*
Surface Properties
Grant Support
ID/Acronym/Agency:
HL-24046/HL/NHLBI NIH HHS; HL-47179/HL/NHLBI NIH HHS
Chemical
Reg. No./Substance:
0/Biocompatible Materials; 0/Dimethylpolysiloxanes; 0/Silanes; 0/Silicones; 63148-62-9/baysilon; 9001-32-5/Fibrinogen

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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