Document Detail


Stimulation of polyprenyl 4-hydroxybenzoate transferase activity by sodium cholate and 3-[(cholamidopropyl)dimethylammonio]-1-propanesulfonate.
MedLine Citation:
PMID:  16643834     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Polyprenyl 4-hydroxybenzoate transferase (Coq2p) plays a central role in ubiquinone biosynthesis. Coq2p mediates the conjugation of 4-hydroxybenzoate, the benzoquinone ring precursor, with the completed side chain. The activity is most easily assayed by measuring the rate of incorporation of 4-hydroxybenzoate as radiolabeled substrate into polyprenyl 4-hydroxybenzoate. The in vitro assay requires addition of a detergent into the reaction mixture to activate enzyme activity, and Triton X-100 is used for this purpose in the routine assay. We have found that both 3-[(cholamidopropyl)dimethylammonio]-1-propanesulfonate and sodium cholate, but not sodium deoxycholate, lysophosphatidyl choline, or octylglucoside, significantly stimulate the activity over that measured with Triton X-100. High-performance liquid chromatography analysis of lipid extracts revealed that the increase of specific activity resulted in a similar increase in reaction product, this effect is due not merely to a better lipid extraction but also to the actual stimulation of enzyme activity. With our improved method, we were able to measure Coq2p activity with much greater sensitivity in both fresh and frozen/thawed mitochondria and in crude homogenates obtained from cultured cells. Our method will simplify evaluation of Coq2p activity in scarce biological materials, such as cells obtained from human tissue biopsies, and thus it will facilitate the biochemical characterization of ubiquinone deficiencies.
Authors:
María I Burón; María D Hermán; Francisco J Alcaín; José M Villalba
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't     Date:  2006-04-18
Journal Detail:
Title:  Analytical biochemistry     Volume:  353     ISSN:  0003-2697     ISO Abbreviation:  Anal. Biochem.     Publication Date:  2006 Jun 
Date Detail:
Created Date:  2006-05-15     Completed Date:  2006-08-01     Revised Date:  2006-11-15    
Medline Journal Info:
Nlm Unique ID:  0370535     Medline TA:  Anal Biochem     Country:  United States    
Other Details:
Languages:  eng     Pagination:  15-21     Citation Subset:  IM    
Affiliation:
Departamento de Biología Celular, Fisiología e Inmunología, Facultad de Ciencias, Campus Universitario de Rabanales, Edificio Severo Ochoa, Universidad de Córdoba, Spain.
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MeSH Terms
Descriptor/Qualifier:
Alkyl and Aryl Transferases / drug effects*
Animals
Cells, Cultured
Cholic Acids / pharmacology*
Chromatography, High Pressure Liquid
Chromatography, Thin Layer
Detergents / pharmacology*
HL-60 Cells
Humans
Lipids / chemistry
Mitochondria, Liver / enzymology
Octoxynol / pharmacology
Parabens / metabolism
Rats
Sodium Cholate / pharmacology*
Ubiquinone / biosynthesis*
Chemical
Reg. No./Substance:
0/Cholic Acids; 0/Detergents; 0/Lipids; 0/Parabens; 1339-63-5/Ubiquinone; 361-09-1/Sodium Cholate; 75621-03-3/3-((3-cholamidopropyl)dimethylammonium)-1-propanesulfonate; 9002-93-1/Octoxynol; 99-96-7/4-hydroxybenzoic acid; EC 2.5.-/Alkyl and Aryl Transferases; EC 2.5.1.-/4-hydroxybenzoate polyprenyltransferase

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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