Document Detail


Spin-label studies of the sulfhydryl environment in bovine plasma albumin. 1. The N--F transition and acid expansion.
MedLine Citation:
PMID:  26387     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The environment of the sulfhydryl group in plasma albumin was previously characterized by employing spin-labels of varying chain lengths (Hull, H. H., Chang, R., & Kaplan, L. J. (1975) Biochim. Biophys. Acta 400, 132). It was established that the sulfhydryl is in a crevice approximately 10 A deep but this crevice was not identified further. We now report the results of titrating albumin through the acidic conformational transitions while monitoring the electron-spin resonance of the bound nitroxide. With short spin-labels a general change is observed as the pH is lowered but the N--F transition is not discernible. However, with a spin label previously shown to project to the lip on the crevice a clear N--F transition as well as the subsequent acid expansion are observed. These results indicate that the sulfhydryl is in the crevice, formed by the domains of albumin, which opens during the N--F transition. Further results indicate that bound fatty acids do not influence the integrity of the sulfhydryl environment at neutral pH.
Authors:
C N Cornell; L J Kaplan
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Biochemistry     Volume:  17     ISSN:  0006-2960     ISO Abbreviation:  Biochemistry     Publication Date:  1978 May 
Date Detail:
Created Date:  1978-08-28     Completed Date:  1978-08-28     Revised Date:  2008-11-21    
Medline Journal Info:
Nlm Unique ID:  0370623     Medline TA:  Biochemistry     Country:  UNITED STATES    
Other Details:
Languages:  eng     Pagination:  1750-4     Citation Subset:  IM    
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MeSH Terms
Descriptor/Qualifier:
Chemical Phenomena
Chemistry
Cyclic N-Oxides
Electron Spin Resonance Spectroscopy
Hydrogen-Ion Concentration
Maleimides
Protein Conformation
Serum Albumin, Bovine*
Spin Labels
Sulfhydryl Compounds
Chemical
Reg. No./Substance:
0/Cyclic N-Oxides; 0/Maleimides; 0/Serum Albumin, Bovine; 0/Spin Labels; 0/Sulfhydryl Compounds

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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