Document Detail


Size effects and breakdown of the power-law blinking statistics of CdSe nanorods.
MedLine Citation:
PMID:  17718457     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
In this study, the dependence of sample size and light intensity on the fluorescence intermittency of semiconductor nanorods is investigated. We present a model with diffusion-controlled electron-transfer reactions involving anomalous diffusion in energy configuration space. This model leads to a general formula t(-m) exp[-(Gammat)n] for the temporal behavior of blinking statistics, where m and n are related to the time dependence of the spectral diffusion. We reanalyze the experimental data of the long-time bending tail of CdSe nanorods and elucidate the size effects of the bending rates and activation energy.
Authors:
Jau Tang
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't; Research Support, U.S. Gov't, Non-P.H.S.     Date:  2007-08-24
Journal Detail:
Title:  The journal of physical chemistry. A     Volume:  111     ISSN:  1089-5639     ISO Abbreviation:  J Phys Chem A     Publication Date:  2007 Sep 
Date Detail:
Created Date:  2007-09-20     Completed Date:  2007-12-03     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9890903     Medline TA:  J Phys Chem A     Country:  United States    
Other Details:
Languages:  eng     Pagination:  9336-9     Citation Subset:  IM    
Affiliation:
Research Center for Applied Sciences, Academia Sinica, Taipei 115, Taiwan. jautang@gate.sinica.edu.tw
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MeSH Terms
Descriptor/Qualifier:
Algorithms
Cadmium Compounds / chemistry*
Diffusion
Models, Chemical*
Nanotubes / chemistry*
Particle Size
Selenium Compounds / chemistry*
Semiconductors
Chemical
Reg. No./Substance:
0/Cadmium Compounds; 0/Selenium Compounds; 1306-24-7/cadmium selenide

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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