Document Detail


Self-repairing oxetane-substituted chitosan polyurethane networks.
MedLine Citation:
PMID:  19286550     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Polyurethanes have many properties that qualify them as high-performance polymeric materials, but they still suffer from mechanical damage. We report the development of polyurethane networks that exhibit self-repairing characteristics upon exposure to ultraviolet light. The network consists of an oxetane-substituted chitosan precursor incorporated into a two-component polyurethane. Upon mechanical damage of the network, four-member oxetane rings open to create two reactive ends. When exposed to ultraviolet light, chitosan chain scission occurs, which forms crosslinks with the reactive oxetane ends, thus repairing the network. These materials are capable of repairing themselves in less than an hour and can be used in many coatings applications, ranging from transportation to packaging or fashion and biomedical industries.
Authors:
Biswajit Ghosh; Marek W Urban
Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  Science (New York, N.Y.)     Volume:  323     ISSN:  1095-9203     ISO Abbreviation:  Science     Publication Date:  2009 Mar 
Date Detail:
Created Date:  2009-03-16     Completed Date:  2009-04-01     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0404511     Medline TA:  Science     Country:  United States    
Other Details:
Languages:  eng     Pagination:  1458-60     Citation Subset:  IM    
Affiliation:
School of Polymers and High Performance Materials, Shelby F. Thames Polymer Science Research Center, University of Southern Mississippi, Hattiesburg, MS 39406, USA.
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MeSH Terms
Descriptor/Qualifier:
Chitosan / chemistry*
Ethers, Cyclic / chemistry*
Molecular Structure
Polyurethanes / chemistry*
Ultraviolet Rays*
Chemical
Reg. No./Substance:
0/Ethers, Cyclic; 0/Polyurethanes; 503-30-0/oxetane; 9012-76-4/Chitosan

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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