Document Detail


Removal of humic acid using TiO2 photocatalytic process--fractionation and molecular weight characterisation studies.
MedLine Citation:
PMID:  18336863     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The photocatalytic removal of humic acid (HA) using TiO2 under UVA irradiation was examined by monitoring changes in the UV(254) absorbance, dissolved organic carbon (DOC) concentration, apparent molecular weight distribution, and trihalomethane formation potentials (THMFPs) over treatment time. A resin fractionation technique in which the samples were fractionated into four components: very hydrophobic acids (VHA), slightly hydrophobic acids, hydrophilic charged (CHA) and hydrophilic neutral (NEU) was also employed to elucidate the changes in the chemical nature of the HA components during treatment. The UVA/TiO2 process was found to be effective in removing more than 80% DOC and 90% UV(254) absorbance. The THMFPs of samples were decreased to below 20 microg l(-1) after treatments, which demonstrate the potential to meet increasingly stringent regulatory level of trihalomethanes in water. Resin fractionation analysis showed that the VHA fraction was decreased considerably as a result of photocatalytic treatments, forming CHA intermediates which were further degraded with increased irradiation time. The NEU fraction, which comprised of non-UV-absorbing low molecular weight compounds, was found to be the most persistent component.
Authors:
Sanly Liu; May Lim; Rolando Fabris; Christopher Chow; Ken Chiang; Mary Drikas; Rose Amal
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't     Date:  2008-03-11
Journal Detail:
Title:  Chemosphere     Volume:  72     ISSN:  0045-6535     ISO Abbreviation:  Chemosphere     Publication Date:  2008 May 
Date Detail:
Created Date:  2008-05-12     Completed Date:  2008-09-22     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0320657     Medline TA:  Chemosphere     Country:  England    
Other Details:
Languages:  eng     Pagination:  263-71     Citation Subset:  IM    
Affiliation:
ARC Centre of Excellence for Functional Nanomaterials, School of Chemical Sciences and Engineering, The University of New South Wales, Sydney NSW 2052, Australia.
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MeSH Terms
Descriptor/Qualifier:
Catalysis / radiation effects
Chemical Fractionation / methods*
Chromatography, Gel
Humic Substances*
Molecular Weight
Spectrophotometry, Ultraviolet
Titanium / chemistry*
Ultraviolet Rays
Chemical
Reg. No./Substance:
0/Humic Substances; 13463-67-7/titanium dioxide; 7440-32-6/Titanium

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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