Document Detail

Pulse-train photoelectron spectroscopy of electronic and nuclear dynamics in molecules.
MedLine Citation:
PMID:  23625832     Owner:  NLM     Status:  In-Data-Review    
We theoretically study the application of a femtosecond pulse train to simultaneously probe the electronic excitation dynamics and nuclear vibrational motion in the excited-state LiH molecule by means of time-resolved photoelectron spectroscopy. The step-like population transfers caused by continual interaction with a sequence of pulses and refractory periods are shown to give rise to time evolution of the photoelectron kinetic energy distribution as the history of molecular electronic and vibrational states. Such a signal should lead to a novel and direct way to investigate electronic and nuclear simultaneous dynamics involving multiple excited states.
Yasuki Arasaki; Kazuo Takatsuka
Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Chemphyschem : a European journal of chemical physics and physical chemistry     Volume:  14     ISSN:  1439-7641     ISO Abbreviation:  Chemphyschem     Publication Date:  2013 May 
Date Detail:
Created Date:  2013-04-29     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  100954211     Medline TA:  Chemphyschem     Country:  Germany    
Other Details:
Languages:  eng     Pagination:  1387-96     Citation Subset:  IM    
Copyright Information:
Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Department of Basic Science, Graduate School of Arts and Sciences, The University of Tokyo, Komaba, 153-8902, Tokyo (Japan).
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