Document Detail


Pressure-induced insertion of liquid alcohols into graphite oxide structure.
MedLine Citation:
PMID:  19947629     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Abstract/OtherAbstract:
Graphite oxide (GO) immersed in an excess of methanol and ethanol media is found to undergo a phase transformation at about 0.2-0.8 GPa, with an expansion of the unit cell volume by approximately 40%, due to pressure-induced insertion of solvent into interlayer space. The pressure at which the structural expansion occurs does not correlate with the solidification pressure of the alcohol, in contrast to the graphite oxide/water system. The expanded high-pressure phase of GO/ethanol could be quenched back to ambient pressure. Compression of graphite oxide with a 2:1 water/methanol medium revealed a complex anomaly with two steps attributed to insertion of methanol and water at different pressure points.
Authors:
Alexandr V Talyzin; Bertil Sundqvist; Tam?s Szab?; Imre D?k?ny; Vladimir Dmitriev
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Journal of the American Chemical Society     Volume:  131     ISSN:  1520-5126     ISO Abbreviation:  J. Am. Chem. Soc.     Publication Date:  2009 Dec 
Date Detail:
Created Date:  2009-12-23     Completed Date:  2010-03-02     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  7503056     Medline TA:  J Am Chem Soc     Country:  United States    
Other Details:
Languages:  eng     Pagination:  18445-9     Citation Subset:  -    
Affiliation:
Department of Physics, Ume? University, SE-901 87 Ume?, Sweden. Alexandr.talyzin@physics.umu.se
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