Document Detail


Prediction of cytochrome P450 2B6-substrate interactions using pharmacophore ensemble/support vector machine (PhE/SVM) approach.
MedLine Citation:
PMID:  18673154     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
An in silico model for predicting human cytochrome P450 2B6-substrate interactions was generated based on a novel scheme, which was initially devised to predict the hERG liability (reported in Leong, M. K., Chem. Res. Toxicol., 2007, 20, 217.) using pharmacophore ensemble/support vector machine to take into account the protein conformational flexibility while interacting with structurally diverse substrates. This is of critical importance yet never being addressed by any analogue-based molecular modeling studies before. Thirty-seven molecules were chosen from the literature and scrutinized for structural integrity and data consistency, of which 26 were treated as the training set to generate models, which were subject to validation by the other 11 molecules as the test set. The predicted pK(m) values by the final PhE/SVM model were in good agreement with observed values. In addition, this in silico model produced an r(2) of 0.84 and a 10-fold cross-validation q(2) of 0.66 for the training set and an r(2) of 0.87 for the test set, asserting the fact that this PhE/SVM model is an accurate model to predict the human P450 2B6-substrates interactions and can be used as a robust prediction tool to facilitate drug discovery.
Authors:
Max K Leong; Tzu-Hsien Chen
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  Medicinal chemistry (Shāriqah (United Arab Emirates))     Volume:  4     ISSN:  1573-4064     ISO Abbreviation:  -     Publication Date:  2008 Jul 
Date Detail:
Created Date:  2008-08-04     Completed Date:  2008-09-25     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  101240303     Medline TA:  Med Chem     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  396-406     Citation Subset:  IM    
Affiliation:
Department of Chemistry, National Dong Hwa University, Shoufeng, Hualien, Taiwan. leong@mail.ndhu.edu.tw
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MeSH Terms
Descriptor/Qualifier:
Cytochrome P-450 Enzyme System / metabolism*
Humans
Models, Molecular
Molecular Conformation
Structure-Activity Relationship
Substrate Specificity
Chemical
Reg. No./Substance:
9035-51-2/Cytochrome P-450 Enzyme System; EC 1.14.14.1/Cytochrome P-450 2B6, human

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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