Document Detail


Polymeric chitosan-based vesicles for drug delivery.
MedLine Citation:
PMID:  9643437     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
A simple carbohydrate polymer glycol chitosan (degree of polymerization 800 approx.) has been investigated for its ability to form polymeric vesicle drug carriers. The attachment of hydrophobic groups to glycol chitosan should yield an amphiphilic polymer capable of self-assembly into vesicles. Chitosan is used because the membrane-penetration enhancement of chitosan polymers offers the possibility of fabricating a drug delivery system suitable for the oral and intranasal administration of gut-labile molecules. Glycol chitosan modified by attachment of a strategic number of fatty acid pendant groups (11-16 mol%) assembles into unilamellar polymeric vesicles in the presence of cholesterol. These polymeric vesicles are found to be biocompatible and haemocompatible and capable of entrapping water-soluble drugs. By use of an ammonium sulphate gradient bleomycin (MW 1400), for example, can be efficiently loaded on to these polymeric vesicles to yield a bleomycin-to-polymer ratio of 0.5 units mg(-1). Previously polymers were thought to assemble into vesicles only if the polymer backbone was separated from the membrane-forming amphiphile by a hydrophilic side-arm spacer. The hydrophilic spacer was thought to be necessary to decouple the random motion of the polymer backbone from the ordered amphiphiles that make up the vesicle membrane. However, stable polymeric vesicles for use in drug delivery have been prepared from a modified carbohydrate polymer, palmitoyl glycol chitosan, without this specific architecture. These polymeric vesicles efficiently entrap water-soluble drugs.
Authors:
I F Uchegbu; A G Schätzlein; L Tetley; A I Gray; J Sludden; S Siddique; E Mosha
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  The Journal of pharmacy and pharmacology     Volume:  50     ISSN:  0022-3573     ISO Abbreviation:  J. Pharm. Pharmacol.     Publication Date:  1998 May 
Date Detail:
Created Date:  1998-09-21     Completed Date:  1998-09-21     Revised Date:  2004-11-17    
Medline Journal Info:
Nlm Unique ID:  0376363     Medline TA:  J Pharm Pharmacol     Country:  ENGLAND    
Other Details:
Languages:  eng     Pagination:  453-8     Citation Subset:  IM    
Affiliation:
Department of Pharmaceutical Sciences, University of Strathclyde, Glasgow, UK.
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MeSH Terms
Descriptor/Qualifier:
Biocompatible Materials / chemistry*
Biopolymers / chemistry
Chitin / analogs & derivatives*,  chemical synthesis,  chemistry
Chitosan
Drug Delivery Systems*
Spectroscopy, Fourier Transform Infrared
Chemical
Reg. No./Substance:
0/Biocompatible Materials; 0/Biopolymers; 0/palmitoyl glycol chitosan; 1398-61-4/Chitin; 9012-76-4/Chitosan

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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