Document Detail


Palladium-catalyzed intramolecular alpha-arylation of alpha-amino acid esters.
MedLine Citation:
PMID:  11798319     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The Pd-catalyzed intramolecular alpha-arylation of alpha-amino acid esters is described. Starting from readily available amino acids, the synthesis of a variety of isoindolines and tetrahydroisoquinoline carboxylic acid esters has been accomplished. Additionally, fused tricyclic systems can be efficiently prepared from cyclic amino acid esters. Reaction conditions have been found that allow the use of tert-butyl ester and N-(benzyloxycarbonyl) protecting groups.
Authors:
Oliver Gaertzen; Stephen L Buchwald
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't; Research Support, U.S. Gov't, P.H.S.    
Journal Detail:
Title:  The Journal of organic chemistry     Volume:  67     ISSN:  0022-3263     ISO Abbreviation:  J. Org. Chem.     Publication Date:  2002 Jan 
Date Detail:
Created Date:  2002-01-18     Completed Date:  2002-04-02     Revised Date:  2007-11-14    
Medline Journal Info:
Nlm Unique ID:  2985193R     Medline TA:  J Org Chem     Country:  United States    
Other Details:
Languages:  eng     Pagination:  465-75     Citation Subset:  IM    
Affiliation:
Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, USA.
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MeSH Terms
Descriptor/Qualifier:
Amino Acids / chemical synthesis*,  chemistry*
Carboxylic Acids / chemical synthesis,  chemistry
Catalysis
Chromatography, Gas
Cyclization
Esters / chemical synthesis*,  chemistry*
Indoles / chemical synthesis,  chemistry
Isoquinolines / chemical synthesis,  chemistry
Molecular Structure
Nuclear Magnetic Resonance, Biomolecular
Palladium / chemistry*
Spectrophotometry, Infrared
Spectroscopy, Fourier Transform Infrared
Grant Support
ID/Acronym/Agency:
GM46059/GM/NIGMS NIH HHS
Chemical
Reg. No./Substance:
0/Amino Acids; 0/Carboxylic Acids; 0/Esters; 0/Indoles; 0/Isoquinolines; 7440-05-3/Palladium

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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