Document Detail


New type of microfabricated carbon electrodes for high-performance liquid chromatography--amperometric detection of fat-soluble vitamins and antioxidants.
MedLine Citation:
PMID:  18538776     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
This study evaluates performance of thin-film carbon electrodes prepared by physical vapor deposition of the electrode material on a polyetheretherketone substrate and compares their performance with that of a standard type of glassy carbon electrodes for chromatographic detection cell of thin-layer type. Kaempferol, retinol, retinyl acetate, cholecalciferol, alpha-tocopherol and gamma-tocopherol were selected for the study and their respective detection limits were found to be 0.63, 5.84, 5.91, 28.19, 16.80 and 16.11 pg. The calibration plots were linear for at least three orders of magnitude for all of the six analytes selected for evaluation. Hydrodynamic voltammograms are shown for both types of electrodes for the range of working electrode potentials between +0.40 and +1.40 V. Also shown and discussed are plots of signal-to-noise vs. detection potential. The working electrode potential of +1.30 V was found to be required for an improved long-term stability of detection performance and was suitable for the detection of all six analytes.
Authors:
Jun Cheng; Petr Jandik
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Publication Detail:
Type:  Journal Article     Date:  2008-05-24
Journal Detail:
Title:  Journal of chromatography. A     Volume:  1198-1199     ISSN:  0021-9673     ISO Abbreviation:  J Chromatogr A     Publication Date:  2008 Jul 
Date Detail:
Created Date:  2008-06-20     Completed Date:  2008-09-22     Revised Date:  2009-01-15    
Medline Journal Info:
Nlm Unique ID:  9318488     Medline TA:  J Chromatogr A     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  148-53     Citation Subset:  IM    
Affiliation:
Research and Development, Dionex Corporation, 1228 Titan Way, Sunnyvale, CA 94088, USA. jun.cheng@dionex.com
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MeSH Terms
Descriptor/Qualifier:
Antioxidants / analysis,  chemistry*
Carbon / chemistry*
Cholecalciferol / analysis,  chemistry
Chromatography, High Pressure Liquid / instrumentation,  methods*
Electrochemistry
Electrodes
Fats / chemistry
Kaempferols / analysis,  chemistry
Reproducibility of Results
Solubility
Vitamin A / analogs & derivatives,  analysis,  chemistry
Vitamins / analysis,  chemistry*
alpha-Tocopherol / analysis,  chemistry
gamma-Tocopherol / analysis,  chemistry
Chemical
Reg. No./Substance:
0/Antioxidants; 0/Fats; 0/Kaempferols; 0/Vitamins; 0/gamma-Tocopherol; 11103-57-4/Vitamin A; 127-47-9/retinol acetate; 520-18-3/kaempferol; 59-02-9/alpha-Tocopherol; 67-97-0/Cholecalciferol; 7440-44-0/Carbon

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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