Document Detail


A more comprehensive and highly practical solution to enantioselective aldehyde crotylation.
MedLine Citation:
PMID:  21486033     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The enantioselective crotylation of aldehydes with 1,2-diaminochlorocrotylsilane reagents is effectively catalyzed by Sc(OTf)(3). The one significant limitation on the utility of these reagents--substrate scope--has thus been addressed. The net result is the most comprehensive and highly practical method for enantioselective aldehyde crotylation yet advanced.
Authors:
Hyunwoo Kim; Stephen Ho; James L Leighton
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Publication Detail:
Type:  Journal Article; Research Support, N.I.H., Extramural     Date:  2011-04-12
Journal Detail:
Title:  Journal of the American Chemical Society     Volume:  133     ISSN:  1520-5126     ISO Abbreviation:  J. Am. Chem. Soc.     Publication Date:  2011 May 
Date Detail:
Created Date:  2011-04-27     Completed Date:  2011-08-19     Revised Date:  2012-05-07    
Medline Journal Info:
Nlm Unique ID:  7503056     Medline TA:  J Am Chem Soc     Country:  United States    
Other Details:
Languages:  eng     Pagination:  6517-20     Citation Subset:  IM    
Copyright Information:
© 2011 American Chemical Society
Affiliation:
Department of Chemistry, Columbia University, New York, New York 10027, USA.
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MeSH Terms
Descriptor/Qualifier:
Aldehydes / chemistry*
Catalysis
Silanes / chemistry*
Stereoisomerism
Grant Support
ID/Acronym/Agency:
R01 GM058133-11/GM/NIGMS NIH HHS; R01 GM058133-12/GM/NIGMS NIH HHS; R01 GM58133/GM/NIGMS NIH HHS
Chemical
Reg. No./Substance:
0/Aldehydes; 0/Silanes; 0/crotylsilane

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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