Document Detail


Laser-enhanced ionization of mercury atoms in an inert atmosphere with avalanche amplification of the signal.
MedLine Citation:
PMID:  21639354     Owner:  NLM     Status:  In-Data-Review    
Abstract/OtherAbstract:
A new method for laser-enhanced ionization detection of mercury atoms in an inert gas atmosphere is described. The method, which is based on the avalanche amplification of the signal resulting from the ionization from a selected Rydberg level reached by a three-step laser excitation of mercury vapor in a simple quartz cell, can be applied to the determination of this element in various matrices by the use of conventional cold atomization techniques. The overall (collisional + photo) ionization efficiency is investigated at different temperatures, and the avalanche amplification effect is reported for Ar and P-10 gases at atmospheric pressure. It is shown that the amplified signal is related to the number of charges produced in the laser-irradiated volume. Under amplifier noise-limited conditions, a detection limit of ∼15 Hg atoms/laser pulse in the interaction region is estimated.
Authors:
W L Clevenger; O I Matveev; S Cabredo; N Omenetto; B W Smith; J D Winefordner
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Analytical chemistry     Volume:  69     ISSN:  0003-2700     ISO Abbreviation:  Anal. Chem.     Publication Date:  1997 Jul 
Date Detail:
Created Date:  2011-06-06     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0370536     Medline TA:  Anal Chem     Country:  United States    
Other Details:
Languages:  eng     Pagination:  2232-7     Citation Subset:  -    
Affiliation:
Department of Chemistry, University of Florida, Gainesville, Florida 32611-7200.
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