Document Detail


Interaction of water and ammonium in NaHY zeolite as detected by combined IR and gravimetric analysis (AGIR).
MedLine Citation:
PMID:  20617275     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Abstract/OtherAbstract:
Qualitative as well as quantitative information is obtained simultaneously by combining thermogravimetry and operando IR spectroscopy with on line mass spectrometry. A microbalance has been adapted to an infrared reactor cell. The weight and IR spectra of a solid sample can be measured together in real time in operando conditions, in a gas flow at temperature between room temperature and 773 K. Molar absorbance coefficients epsilons can be obtained directly. The new technique was first applied to adsorbed water and ammonia on a solid acid catalyst, HY zeolite. Epsilon coefficients for water bands were measured. They are influence by the hydration level, and the nu+delta combination band is shown to be a much better option to determine the amount of adsorbed water on zeolites. Epsilon has also been measured for ammonium ions, and water was shown to greatly influence the spectral response of these ions.
Authors:
Philippe Bazin; Aurélie Alenda; Frédéric Thibault-Starzyk
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Publication Detail:
Type:  Journal Article     Date:  2010-07-09
Journal Detail:
Title:  Dalton transactions (Cambridge, England : 2003)     Volume:  39     ISSN:  1477-9234     ISO Abbreviation:  Dalton Trans     Publication Date:  2010 Sep 
Date Detail:
Created Date:  2010-09-02     Completed Date:  2010-12-14     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  101176026     Medline TA:  Dalton Trans     Country:  England    
Other Details:
Languages:  eng     Pagination:  8432-6     Citation Subset:  -    
Affiliation:
Laboratoire Catalyse et Spectrochimie, ENSICAEN-Université de Caen-CNRS, 6 Boulevard Maréchal Juin, 14050, Caen, France. philippe.bazin@ensicaen.fr
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