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Influence of dendrimer generation and polyethylene glycol length on the biodistribution of PEGylated dendrimers.
MedLine Citation:
PMID:  19761822     Owner:  NLM     Status:  In-Process    
Abstract/OtherAbstract:
Dendrimers are a potential drug carrier. Because modification with polyethylene glycol (PEG) is known to improve the blood retention, PEGylated dendrimers have been studied as a useful drug carrier. In this study, three types of PEGylated L-lysine-bearing polyamidoamine dendrimers (PEG2k-Lys-PAMAM (G4), PEG5k-Lys-PAMAM (G4), PEG2k-Lys-PAMAM (G5)) were synthesized, which are composed of a dendrimer of different generations (generations 4 and 5) and PEG chains with different molecular weights (2k and 5k). An acetylated L-lysine-bearing dendrimer was also synthesized as a non-PEGylated dendrimer. Bifunctional diethylenetriaminepentaacetic acid (pSCN-benzyl-DTPA) was bound to the epsilon -amino group of lysine in a dendrimer, to be labeled with radioactive indium-111. These PEGylayed dendrimers showed longer blood retention and lower accumulation in other normal organs such as the kidneys than the non-PEGylated dendrimer. The PEGylated dendrimers with the higher generation and the longer PEG led the greater blood retention.
Authors:
Chie Kojima; Celeste Regino; Yasuhito Umeda; Hisataka Kobayashi; Kenji Kono
Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't     Date:  2009-09-15
Journal Detail:
Title:  International journal of pharmaceutics     Volume:  383     ISSN:  1873-3476     ISO Abbreviation:  Int J Pharm     Publication Date:  2010 Jan 
Date Detail:
Created Date:  2009-11-25     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  7804127     Medline TA:  Int J Pharm     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  293-6     Citation Subset:  IM    
Affiliation:
Department of Applied Chemistry, Graduate School of Engineering, Osaka Prefecture University, Osaka, Japan. c-kojima@21c.osakafu-u.ac.jp
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