Document Detail


Highly Efficient Ultrafast Electron Injection from the Singlet MLCT Excited State of Copper(I) Diimine Complexes to TiO(2) Nanoparticles.
MedLine Citation:
PMID:  23136096     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
Cu complex as photosensitizers: Photoinduced charge-transfer dynamics from a copper(I) diimine complex to TiO(2) nanoparticles were investigated by combining multiple time-resolved spectroscopic methods. An efficient and ultrafast electron transfer process from the singlet MLCT state was discovered as a result of structural control owing to the flattening of the tetrahedral geometry in the complex and the bulky groups in the ligands.
Authors:
Jier Huang; Onur Buyukcakir; Michael W Mara; Ali Coskun; Nada M Dimitrijevic; Gokhan Barin; Oleksandr Kokhan; Andrew B Stickrath; Romain Ruppert; David M Tiede; J Fraser Stoddart; Jean-Pierre Sauvage; Lin X Chen
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Publication Detail:
Type:  JOURNAL ARTICLE     Date:  2012-11-8
Journal Detail:
Title:  Angewandte Chemie (International ed. in English)     Volume:  -     ISSN:  1521-3773     ISO Abbreviation:  Angew. Chem. Int. Ed. Engl.     Publication Date:  2012 Nov 
Date Detail:
Created Date:  2012-11-8     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0370543     Medline TA:  Angew Chem Int Ed Engl     Country:  -    
Other Details:
Languages:  ENG     Pagination:  -     Citation Subset:  -    
Copyright Information:
Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Affiliation:
Chemical Sciences and Engineering Argonne National Laboratory, Argonne, IL 60439 (USA).
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