Document Detail


High-Pressure Scanning Tunneling Microscopy of a Silver Surface during Catalytic Formation of Ethylene Oxide.
MedLine Citation:
PMID:  23592599     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
The active state of a catalyst: A high-pressure scanning tunneling microscope (STM) was used to bridge the pressure gap for the Ag-catalyzed ethylene epoxidation. An active oxygen species on an Ag(111) single crystal was characterized under ultra-high vacuum conditions. The same species was identified with STM in an ethylene/oxygen mixture. In the STM cell the formation of ethylene oxide was detected.
Authors:
Sebastian Böcklein; Sebastian Günther; Joost Wintterlin
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Publication Detail:
Type:  JOURNAL ARTICLE     Date:  2013-4-16
Journal Detail:
Title:  Angewandte Chemie (International ed. in English)     Volume:  -     ISSN:  1521-3773     ISO Abbreviation:  Angew. Chem. Int. Ed. Engl.     Publication Date:  2013 Apr 
Date Detail:
Created Date:  2013-4-17     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0370543     Medline TA:  Angew Chem Int Ed Engl     Country:  -    
Other Details:
Languages:  ENG     Pagination:  -     Citation Subset:  -    
Copyright Information:
Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Affiliation:
Department Chemie, Ludwig-Maximilians-Universität München, Butenandtstr. 5-13, 81377 Munich (Germany) http://physchem.cup.uni-muenchen.de/wintterlin/
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