Document Detail


Hierarchical Dynamics of Correlated System-Environment Coherence and Optical Spectroscopy.
MedLine Citation:
PMID:  21452824     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
We propose an efficient construction of the hierarchical equations of motion formalism of quantum dissipation on the basis of the Padé spectrum decomposition of the Bose function and the multiple Brownian oscillators decomposition of the environment spectral density. The related hierarchical Liouville space algebra for quantum dissipative mechanics is outlined in relation to the evaluation of nonlinear optical response functions. With the simulated transient pump-probe spectroscopy of model exciton systems, we demonstrate the correlated system-environment coherence by the present nonperturbative and non-Markovian quantum dissipation theory.
Authors:
Kun-Bo Zhu; Rui-Xue Xu; Hou Yu Zhang; Jie Hu; Yi Jing Yan
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Publication Detail:
Type:  JOURNAL ARTICLE     Date:  2011-3-31
Journal Detail:
Title:  The journal of physical chemistry. B     Volume:  -     ISSN:  1520-5207     ISO Abbreviation:  -     Publication Date:  2011 Mar 
Date Detail:
Created Date:  2011-4-1     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  101157530     Medline TA:  J Phys Chem B     Country:  -    
Other Details:
Languages:  ENG     Pagination:  -     Citation Subset:  -    
Affiliation:
State Key Laboratory of Supramolecular Structure and Materials, Jilin University , Changchun 130012, China.
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