Document Detail


Fast-atom bombardment and thermospray mass spectrometry for the characterization of two glucuronide metabolites of methapyrilene.
MedLine Citation:
PMID:  2520227     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Two conjugated metabolites of methapyrilene hydrochloride isolated from mouse-hepatocytes were examined by mass spectrometry using fast-atom bombardment (FAB) and thermospray ionization. The major metabolite, methapyrilene glucuronide, was identified based on a prominent peak due to the protonated molecule as well as the loss of the dimethylamine and sugar moieties. Identification of the second metabolite was complicated by large signals associated with the biological sample matrix. The complementary nature of the fragmentation observed in the mass spectra using FAB and thermospray ionization allowed this metabolite to be identified as the desmethylmethapyrilene glucuronide. The fragmentation observed using FAB ionization was not greatly affected by the presence of the glucuronide moiety. While loss of the sugar moiety indicated a glucuronide, additional fragmentation confirmed the presence of the underlying ethylenediamine substructure which is characteristic of this class of antihistamines.
Authors:
J O Lay; T A Getek; D W Kelly; W Slikker; W A Korfmacher
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Publication Detail:
Type:  In Vitro; Journal Article    
Journal Detail:
Title:  Rapid communications in mass spectrometry : RCM     Volume:  3     ISSN:  0951-4198     ISO Abbreviation:  Rapid Commun. Mass Spectrom.     Publication Date:  1989 Mar 
Date Detail:
Created Date:  1992-04-24     Completed Date:  1992-04-24     Revised Date:  2006-11-15    
Medline Journal Info:
Nlm Unique ID:  8802365     Medline TA:  Rapid Commun Mass Spectrom     Country:  ENGLAND    
Other Details:
Languages:  eng     Pagination:  72-5     Citation Subset:  IM    
Affiliation:
Food and Drug Administration, National Center for Toxicological Research, Jefferson, Arkansas 72079.
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MeSH Terms
Descriptor/Qualifier:
Animals
Glucuronates / analysis*
Liver / metabolism*
Mass Spectrometry / methods
Methapyrilene / analogs & derivatives*,  analysis*
Mice
Spectrometry, Mass, Fast Atom Bombardment / methods
Chemical
Reg. No./Substance:
0/Glucuronates; 91-80-5/Methapyrilene

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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