Document Detail


Exchange-coupled cobalt(II) dimer with unusual magnetic circular dichroism saturation behavior.
MedLine Citation:
PMID:  20608659     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Abstract/OtherAbstract:
The exchange-coupled complex [Co(2)(mu-H(2)O)(mu-OAc)(2)(OAc)(2)(tmen)(2)] (OAc = CH(3)COO(-) acetato; tmen = N,N,N',N'-tetramethylenediamine) has been studied by magnetic circular dichroism (MCD) spectroscopy and magnetization measurements. A peculiar behavior of the MCD spectra was observed with a change in the magnetic field. The intensity of particular lines initially increases, then decreases with an increase in the magnetic field strength, disappears with a further field increase, and appears again with the opposite sign. This behavior was explained by the overlap of the electronic transitions at different but near wavelengths. The obtained MCD magnetization curves, together with magnetization obtained by a SQUID magnetometer, are well reproduced using the Hamiltonian, which takes into account an orbital magnetic moment.
Authors:
S Ostrovsky; Z Tomkowicz; W Haase
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Inorganic chemistry     Volume:  49     ISSN:  1520-510X     ISO Abbreviation:  Inorg Chem     Publication Date:  2010 Aug 
Date Detail:
Created Date:  2010-07-29     Completed Date:  2010-11-23     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0366543     Medline TA:  Inorg Chem     Country:  United States    
Other Details:
Languages:  eng     Pagination:  6942-7     Citation Subset:  -    
Affiliation:
Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Darmstadt University of Technology, Petersenstrasse 20, 64287 Darmstadt, Germany.
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