Document Detail


Evidence of chemical bonding to hydroxyapatite by phosphoric acid esters.
MedLine Citation:
PMID:  15792536     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Phosphoric acid esters (PAEs) have been used as a self-etching primer for composite-to-enamel bonding in adhesive dentistry. However, the chemical mechanism of their interactions with hydroxyapatite (HA) is not clear. In the present study, HA particles were mixed with Resulcin AquaPrime (Merz Co.) priming agent that contains a mixture of PAEs, and dried. The primer, HA and the mixture of both were analyzed by FTIR. Primed and untreated HA discs were analyzed with attenuated total reflectance (ATR). After AquaPrime+D(2)O (1:1) was mixed with HA or Ca(OD)(2) for 48 h, the primer and both mixtures were analyzed with (31)P NMR in D(2)O. The solid and the liquid separated from both mixtures were analyzed with (31)P NMR in CDCl(3). The primer's characteristic bands (nu(CO), nu(CC)) were found on the primer-subtracted mixture's spectrum and the primed HA disc. (31)P NMR data indicated that the reactions of PAEs with HA produced PAEs-HA complexes, and were not a simple acid-base reaction like those with Ca(OD)(2), either in liquid or in solid. It is concluded that phosphoric acid esters can decalcify and adhere to hydroxyapatite simultaneously.
Authors:
Baiping Fu; Xuemei Sun; Weixin Qian; Yanqing Shen; Ranran Chen; Matthias Hannig
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Biomaterials     Volume:  26     ISSN:  0142-9612     ISO Abbreviation:  Biomaterials     Publication Date:  2005 Sep 
Date Detail:
Created Date:  2005-03-28     Completed Date:  2005-09-06     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  8100316     Medline TA:  Biomaterials     Country:  England    
Other Details:
Languages:  eng     Pagination:  5104-10     Citation Subset:  IM    
Affiliation:
Department of Stomatology, No. 1 Hospital affiliated to Medical College, Zhejiang University, Hangzhou 310003, China. baipingfu@hotmail.com
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MeSH Terms
Descriptor/Qualifier:
Acid Etching, Dental
Calcium / chemistry
Dentin-Bonding Agents / chemistry
Durapatite / chemistry*
Humans
Magnetic Resonance Spectroscopy
Phosphoric Acid Esters / chemistry*
Spectrophotometry, Infrared
Spectroscopy, Fourier Transform Infrared
Surface Properties
Chemical
Reg. No./Substance:
0/Dentin-Bonding Agents; 0/Phosphoric Acid Esters; 1306-06-5/Durapatite; 7440-70-2/Calcium

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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