Document Detail


Evaluation of 'east-to-west' ether-forming strategies for the total synthesis of maoecrystal V.
MedLine Citation:
PMID:  23316095     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
Model systems that evaluated different approaches to construct the central ether ring of maoecrystal V are described. Our first model systems attempted the ether formation using C-H functionalization reactions, which led to interesting rearrangements but none of the desired ether product. An intramolecular conjugate addition strategy was then explored that successfully formed the targeted C-O bond but resulted in the undesired stereochemistry.
Authors:
Kiel E Lazarski; Berkcan Akpinar; Regan J Thomson
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Publication Detail:
Type:  JOURNAL ARTICLE    
Journal Detail:
Title:  Tetrahedron letters     Volume:  54     ISSN:  0040-4039     ISO Abbreviation:  Tetrahedron Lett.     Publication Date:  2013 Feb 
Date Detail:
Created Date:  2013-1-14     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  2984819R     Medline TA:  Tetrahedron Lett     Country:  -    
Other Details:
Languages:  ENG     Pagination:  635-637     Citation Subset:  -    
Affiliation:
Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208.
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