Document Detail


Enantioseparation of amino acids, alpha-hydroxy acids, and dipeptides by ligand-exchange CEC using silica-based chiral stationary phases.
MedLine Citation:
PMID:  19655330     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
This work deals with the application of silica-based ligand-exchange chiral stationary phases (CSPs) for the enantioseparation of underivatized amino acids, alpha-hydroxy acids, and dipeptides with packed CEC. Two different possibilities of preparing silica-based CSPs are presented. One phase contains L-4-hydroxyproline chemically bonded via a spacer to 3 mum silica material. The other approach makes use of N-decyl-L-4-hydroxyproline dynamically coated on a reversed-phase packed capillary. Dynamical coating of reversed-phase material represents a simple alternative to prepare CSP. A comparison of the chemically bonded phase with the dynamically coated CSP by means of resolution of complex-forming analytes is presented. The chemically bonded phase was found to be superior to the dynamically coated phase in terms of resolution of amino acids and dipeptides. However, the dynamically coated CSP was found to be especially suitable for the separation of alpha-hydroxy acids. Both techniques are applicable for enantiomer purity tests.
Authors:
Elfriede Pittler; Nina Grawatsch; D??rte Paul; Gerald G??bitz; Martin G Schmid
Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Electrophoresis     Volume:  30     ISSN:  1522-2683     ISO Abbreviation:  Electrophoresis     Publication Date:  2009 Aug 
Date Detail:
Created Date:  2009-08-26     Completed Date:  2010-01-05     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  8204476     Medline TA:  Electrophoresis     Country:  Germany    
Other Details:
Languages:  eng     Pagination:  2897-904     Citation Subset:  IM    
Affiliation:
Institute of Pharmaceutical Sciences, Department of Pharmaceutical Chemistry, Karl-Franzens-University, Austria.
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MeSH Terms
Descriptor/Qualifier:
Amino Acids / isolation & purification*
Capillary Electrochromatography / methods*
Dipeptides / isolation & purification*
Hydrogen-Ion Concentration
Hydroxy Acids / isolation & purification*
Ligands
Phenylalanine / analogs & derivatives,  isolation & purification
Silicon Dioxide / chemistry*
Stereoisomerism
Temperature
Chemical
Reg. No./Substance:
0/Amino Acids; 0/Dipeptides; 0/Hydroxy Acids; 0/Ligands; 325-69-9/2-fluorophenylalanine; 63-91-2/Phenylalanine; 7631-86-9/Silicon Dioxide

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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