Document Detail


Efficient synthesis of omega-mercaptoalkyl 1,2-trans-glycosides from sugar peracetates.
MedLine Citation:
PMID:  17362892     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Lewis acid-promoted reactions of peracetylated sugars (glucose, galactose, maltose, lactose) with omega-bromo-1-alkanols (C(8), C(12)) were investigated. ZnCl(2) was found to promote the 1,2-trans-glycosylation of the alcohols in toluene at about 60 degrees C in a stereocontrolled manner with better yields than commonly employed promoters such as SnCl(4). The omega-bromoalkyl acetylated glycosides were readily converted to omega-mercaptoalkyl glycosides, which are useful for the preparation of glycoclusters.
Authors:
Teiichi Murakami; Reiko Hirono; Yukari Sato; Kiyotaka Furusawa
Publication Detail:
Type:  Journal Article     Date:  2007-02-25
Journal Detail:
Title:  Carbohydrate research     Volume:  342     ISSN:  0008-6215     ISO Abbreviation:  Carbohydr. Res.     Publication Date:  2007 Jun 
Date Detail:
Created Date:  2007-04-16     Completed Date:  2007-08-01     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  0043535     Medline TA:  Carbohydr Res     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  1009-20     Citation Subset:  IM    
Affiliation:
Institute for Biological Resources and Functions, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba Central 5, Tsukuba, Ibaraki 305-8565, Japan. t-murakami@aist.go.jp
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MeSH Terms
Descriptor/Qualifier:
Acetates*
Acetylation
Alcohols / metabolism
Carbohydrate Conformation
Carbohydrates / chemistry
Disaccharides / chemical synthesis,  chemistry
Glucose / chemistry
Glycosides / chemical synthesis*
Glycosylation
Hexoses / metabolism*
Models, Molecular
Oligosaccharides / chemical synthesis
Proteins / chemistry
Chemical
Reg. No./Substance:
0/Acetates; 0/Alcohols; 0/Carbohydrates; 0/Disaccharides; 0/Glycosides; 0/Hexoses; 0/Oligosaccharides; 0/Proteins; 50-99-7/Glucose

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