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Efficiency-improved organic solar cells based on plasticizer assisted soft embossed PEDOT:PSS layers.
MedLine Citation:
PMID:  23038272     Owner:  NLM     Status:  Publisher    
Abstract/OtherAbstract:
Organic solar cells (OSCs) have attracted extensive attention as a promising approach for cost-effective photovoltaic devices. This study demonstrates a novel imprinting approach based on additional plasticizing, which is suited for thin polyethylenedioxythiophene:polystyrenesulphonate (PEDOT:PSS) layers. Such films are widely used as electron blocking and hole collecting intermediate layers in OSCs. Master molds with nano-scale channels are used for the temperature and pressure assisted imprinting routine and the shape of the imprinted structures is easily tunable via the plasticizer concentration. Depending on the surface topology of the PEDOT:PSS films structured poly(3-hexylthiophene) (P3HT):phenyl-C(61)-butyric acid methyl ester (PCBM) bulk heterojunction solar cells have improved power conversion efficiencies in comparison to their planar references. This effect results from enhanced optical absorption due to the resulting textured aluminum electrode and improved charge carrier extraction at the artificially structured electrodes. In addition, OSCs based on low aspect ratio PEDOT:PSS imprints show increased relative performance under oblique light incidence.
Authors:
Robert Meier; Christopher Birkenstock; Claudia M Palumbiny; Peter Müller-Buschbaum
Publication Detail:
Type:  JOURNAL ARTICLE     Date:  2012-10-4
Journal Detail:
Title:  Physical chemistry chemical physics : PCCP     Volume:  -     ISSN:  1463-9084     ISO Abbreviation:  Phys Chem Chem Phys     Publication Date:  2012 Oct 
Date Detail:
Created Date:  2012-10-5     Completed Date:  -     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  100888160     Medline TA:  Phys Chem Chem Phys     Country:  -    
Other Details:
Languages:  ENG     Pagination:  -     Citation Subset:  -    
Affiliation:
Technische Universität München, Physik-Department, Lehrstuhl für Funktionelle Materialien, James-Franck-Str. 1, 85748 Garching, Germany. muellerb@ph.tum.de.
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