Document Detail


Effects of the novel Foxo1 inhibitor AS1708727 on plasma glucose and triglyceride levels in diabetic db/db mice.
MedLine Citation:
PMID:  20655898     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Recent evidence suggests that the forkhead transcription factor Foxo1 plays an important role in the regulation of glucose and triglyceride metabolism at the gene transcription level for glucose-6 phosphatase (G6Pase), phosphoenolpyruvate carboxykinase (PEPCK), and apolipoprotein C-III (apoC-III). Here, we report on the pharmacological effects of the novel Foxo1 inhibitor AS1708727, which we identified by compound screening. Chronic treatment of diabetic db/db mice with AS1708727 for four days significantly reduced blood glucose and triglyceride levels with decrease of gene expression levels of hepatic G6Pase, PEPCK, and apoC-III. No reports have yet examined the influence of Foxo1 inhibitors on these pharmacological effects. In this study, we newly identified a Foxo1 inhibitor compound capable of exerting both an anti-hypertriglyceridemic and anti-hyperglycemic effect. These effects were dependent on maintaining a stable blood concentration of AS1708727 and achieving a high rate of compound transition to the liver. We also investigated the action mechanism of AS1708727 on gluconeogenesis in vitro and in vivo. The compound inhibited gene expression of key gluconeogenic molecules and suppressed gluconeogenesis in Fao hepatocyte cells in vitro. Further, in the pyruvate challenge study using db/db mice in vivo, AS1708727 suppressed increases in blood glucose level by inhibiting gluconeogenic gene expression. These results indicate that the novel Foxo1 inhibitor AS1708727 may exert anti-diabetic and anti-hypertriglyceridemic effects by improving blood glucose and triglyceride metabolism at the gene expression level, and may represent a new class of drugs useful for treating type 2 diabetes mellitus and hypertriglyceridemia.
Authors:
Hirotsugu Tanaka; Takeyuki Nagashima; Akiyoshi Shimaya; Yasuharu Urano; Teruhiko Shimokawa; Masayuki Shibasaki
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Publication Detail:
Type:  Journal Article     Date:  2010-07-23
Journal Detail:
Title:  European journal of pharmacology     Volume:  645     ISSN:  1879-0712     ISO Abbreviation:  Eur. J. Pharmacol.     Publication Date:  2010 Oct 
Date Detail:
Created Date:  2010-08-30     Completed Date:  2011-01-19     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  1254354     Medline TA:  Eur J Pharmacol     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  185-91     Citation Subset:  IM    
Copyright Information:
Copyright 2010 Elsevier B.V. All rights reserved.
Affiliation:
Pharmacology Research Labs, Drug Discovery Research, Astellas Pharma Inc., 21 Miyukigaoka, Tuskuba, Ibaraki 305-8585, Japan. hirotsugu.tanaka@jp.astellas.com
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MeSH Terms
Descriptor/Qualifier:
Acetanilides / pharmacokinetics*
Animals
Apolipoprotein C-III / metabolism
Blood Glucose / metabolism*
Cells, Cultured
Diabetes Mellitus, Type 2 / metabolism*
Forkhead Transcription Factors / antagonists & inhibitors*
Gluconeogenesis
Glucose-6-Phosphatase / metabolism
Hepatocytes / drug effects,  metabolism
Hypertriglyceridemia / metabolism
Hypoglycemic Agents / pharmacology*
Hypolipidemic Agents / pharmacology*
Isoquinolines / pharmacokinetics*
Male
Mice
Mice, Inbred C57BL
Phosphoenolpyruvate Carboxykinase (GTP) / metabolism
Triglycerides / blood*
Chemical
Reg. No./Substance:
0/2-cyclopentyl-N-(2,4-dichloro-3-((isoquinolin-5-yloxy)methyl)phenyl)-N-methylacetamide; 0/Acetanilides; 0/Apolipoprotein C-III; 0/Blood Glucose; 0/Forkhead Transcription Factors; 0/Foxo1 protein, mouse; 0/Hypoglycemic Agents; 0/Hypolipidemic Agents; 0/Isoquinolines; 0/Triglycerides; EC 3.1.3.9/Glucose-6-Phosphatase; EC 4.1.1.32/Phosphoenolpyruvate Carboxykinase (GTP)

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