Document Detail


Discovery and pharmacological characterization of aryl piperazine and piperidine ethers as dual acting norepinephrine reuptake inhibitors and 5-HT1A partial agonists.
MedLine Citation:
PMID:  19854053     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Compounds that are both norepinephrine reuptake inhibitors (NRI) and 5-HT1(A) partial agonists may have the potential to treat neuropsychiatric disorders including attention deficit hyperactivity disorder (ADHD) and depression. Targeted screening of NRI-active compounds for binding to the 5-HT(1A) receptor provided a series of thiomorpholinone hits with this dual activity profile. Several iterations of design, synthesis, and testing led to substituted piperidine diphenyl ethers which are potent NRIs with 5-HT1(A) partial agonist properties. In addition, optimization of these molecules provided compounds which exhibit selectivity for NRI over the dopamine (DAT) and serotonin (SERT) reuptake transporters. Monoamine and 5-HT(1A) in vitro functional activities for select compounds from the developed piperidine diphenyl ether series are also presented.
Authors:
David L Gray; Wenjian Xu; Brian M Campbell; Amy B Dounay; Nancy Barta; Susan Boroski; Lynne Denny; Lori Evans; Nancy Stratman; Al Probert
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Publication Detail:
Type:  Journal Article     Date:  2009-10-12
Journal Detail:
Title:  Bioorganic & medicinal chemistry letters     Volume:  19     ISSN:  1464-3405     ISO Abbreviation:  Bioorg. Med. Chem. Lett.     Publication Date:  2009 Dec 
Date Detail:
Created Date:  2009-11-05     Completed Date:  2010-01-19     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  9107377     Medline TA:  Bioorg Med Chem Lett     Country:  England    
Other Details:
Languages:  eng     Pagination:  6604-7     Citation Subset:  IM    
Affiliation:
Pfizer Global Research and Development, Eastern Point Road, Groton, CT 06340, United States. david.l.gray@pfizer.com
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MeSH Terms
Descriptor/Qualifier:
Dopamine / metabolism
Drug Discovery*
Ethers / chemical synthesis,  chemistry,  pharmacology*
Molecular Structure
Neurotransmitter Uptake Inhibitors / chemical synthesis,  chemistry,  pharmacology*
Piperazines / chemical synthesis,  chemistry,  pharmacology*
Piperidines / chemical synthesis,  chemistry,  pharmacology*
Receptor, Serotonin, 5-HT1A / agonists*
Serotonin Plasma Membrane Transport Proteins / metabolism
Stereoisomerism
Structure-Activity Relationship
Chemical
Reg. No./Substance:
0/Ethers; 0/Neurotransmitter Uptake Inhibitors; 0/Piperazines; 0/Piperidines; 0/Serotonin Plasma Membrane Transport Proteins; 112692-38-3/Receptor, Serotonin, 5-HT1A

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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