Document Detail


Differential effects of cyclodextrins and derivatives on the biological behavior of the myocardial perfusion imaging agent 99mTcN-NOET.
MedLine Citation:
PMID:  16000249     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
In addition to improving drug solubilization, cyclodextrins (CDs) also affect the biological behavior of the included compound. We evaluated the effects of two natural CDs beta-CD and gamma-CD, and six beta-CD derivatives, Dimeb, Trimeb, SBb, 2-HP, 6AD, and 6 MTU on the biological behavior of (99m)TcN-NOET, a technetium-99m-labeled, lipophilic compound readily detectable through radioactivity assessment. Determination of CDs' affinities for (99m)TcN-NOET indicated that the cavity size of gamma-CD was not suitable for (99m)TcN-NOET inclusion, and that beta-CD derivatization mostly resulted in decreased CDs affinities for (99m)TcN-NOET to various extents compared with the natural beta-CD. In vitro and ex vivo experiments performed on newborn rat cardiomyocytes and isolated perfused rat hearts, respectively, showed 1.7- and 2.3-fold maximal differences in (99m)TcN-NOET cellular and tissue activities. Regression analyzes indicated no significant correlation between these observed biological differences and the affinities of the eight CDs tested for (99m)TcN-NOET or for cellular membranes. In conclusion, CD derivatization often resulted in impaired affinity of the derivatives for the lipophilic compound (99m)TcN-NOET. Moreover, the in vitro and ex vivo biological behavior of (99m)TcN-NOET was greatly affected depending on the CD used for inclusion of the tracer.
Authors:
Laurent Riou; Catherine Ghezzi; Denis Wouessidjewe; Ho Law; Jean-Paul Mathieu; Jacques Defaye; René Bontron; Roberto Pasqualini; Daniel Fagret
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Publication Detail:
Type:  In Vitro; Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  European journal of pharmaceutics and biopharmaceutics : official journal of Arbeitsgemeinschaft für Pharmazeutische Verfahrenstechnik e.V     Volume:  61     ISSN:  0939-6411     ISO Abbreviation:  Eur J Pharm Biopharm     Publication Date:  2005 Sep 
Date Detail:
Created Date:  2005-08-08     Completed Date:  2005-11-10     Revised Date:  2006-11-15    
Medline Journal Info:
Nlm Unique ID:  9109778     Medline TA:  Eur J Pharm Biopharm     Country:  Netherlands    
Other Details:
Languages:  eng     Pagination:  40-9     Citation Subset:  IM    
Affiliation:
INSERM E0340 Radiopharmaceutiques Biocliniques, Faculté de Médecine de Grenoble, Domaine de la Merci, La Tronche, France. laurent.riou@ujf-grenoble.fr
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MeSH Terms
Descriptor/Qualifier:
Animals
Animals, Newborn
Cyclodextrins / chemistry*,  pharmacokinetics
Dogs
Heart / radionuclide imaging*
Linear Models
Male
Myocardium / metabolism*
Myocytes, Cardiac / metabolism*
Organotechnetium Compounds / chemistry,  pharmacokinetics*
Rats
Rats, Wistar
Solubility
Thiocarbamates / chemistry,  pharmacokinetics*
Chemical
Reg. No./Substance:
0/Cyclodextrins; 0/Organotechnetium Compounds; 0/Thiocarbamates; 0/technetium Tc 99m, bis(N-ethoxy-N-ethyldithiocarbamato)nitrido-

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