Document Detail


Deconvolution of isobaric interferences in mass spectra.
MedLine Citation:
PMID:  15121194     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The concept of isobar deconvolution using the mass domain and signal intensity based domains is described. The intensity domain-based approach employs the reconstruction of the observed isotope pattern from the isolated patterns of the isobaric species. The quantitative information is adjusted with the use of the least squares algorithm. The mass domain-based approach employs signal deconvolution by forming Gaussian components for which the peak width and position can be predicted a priori. The latter method is applicable to medium resolution instruments, such as TOF-MS, while the pattern reconstruction approach is applicable also to low resolution instrumentation, such as quadrupole-based ICP-MS or GC/MS. An example of CH(z)Se (z = 0-4) cluster analysis in dimethyl diselenide mass spectra is given to illustrate the concepts underlying both approaches.
Authors:
Juris Meija; Joseph A Caruso
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Publication Detail:
Type:  Journal Article; Research Support, U.S. Gov't, P.H.S.    
Journal Detail:
Title:  Journal of the American Society for Mass Spectrometry     Volume:  15     ISSN:  1044-0305     ISO Abbreviation:  J. Am. Soc. Mass Spectrom.     Publication Date:  2004 May 
Date Detail:
Created Date:  2004-05-03     Completed Date:  2004-06-18     Revised Date:  2007-11-14    
Medline Journal Info:
Nlm Unique ID:  9010412     Medline TA:  J Am Soc Mass Spectrom     Country:  United States    
Other Details:
Languages:  eng     Pagination:  654-8     Citation Subset:  IM    
Affiliation:
Department of Chemistry, University of Cincinnati, Cincinnati, Ohio 45221-0172, USA.
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MeSH Terms
Descriptor/Qualifier:
Algorithms
Isotopes
Mass Spectrometry / methods*
Models, Molecular
Sensitivity and Specificity
Grant Support
ID/Acronym/Agency:
ES04908/ES/NIEHS NIH HHS
Chemical
Reg. No./Substance:
0/Isotopes

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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