Document Detail


Cooperativity in the binding of the cationic biocide polyhexamethylene biguanide to nucleic acids.
MedLine Citation:
PMID:  15120614     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
The interaction between the broad-spectrum antimicrobial agent, polyhexamethylene biguanide (PHMB), and various nucleic acids was investigated. Titration of either single- or double-stranded 100-bp DNA, or mixed-molecular weight marker DNA, or tRNA with PHMB caused precipitation of a complex between nucleic acid and PHMB in which the nucleotide/biguanide ratio was always close to unity. Binding of PHMB was highly cooperative, with apparent Hill coefficients 10.3-14.6. When a fluorescent derivative of PHMB was titrated with increasing amounts of nucleic acid, all four forms of nucleic acid caused strong polarisation of fluorescence, demonstrating the association with PHMB. The intensity and broad-spectrum binding of PHMB to all forms of nucleic acid has significant implications for the mechanism of action of this biocide.
Authors:
Michael J Allen; Andrew P Morby; Graham F White
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Biochemical and biophysical research communications     Volume:  318     ISSN:  0006-291X     ISO Abbreviation:  Biochem. Biophys. Res. Commun.     Publication Date:  2004 May 
Date Detail:
Created Date:  2004-05-03     Completed Date:  2004-06-25     Revised Date:  2009-11-19    
Medline Journal Info:
Nlm Unique ID:  0372516     Medline TA:  Biochem Biophys Res Commun     Country:  United States    
Other Details:
Languages:  eng     Pagination:  397-404     Citation Subset:  IM    
Affiliation:
Cardiff School of Biosciences, Cardiff University, Cardiff CF10 3US, UK.
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MeSH Terms
Descriptor/Qualifier:
Anti-Infective Agents / chemistry,  metabolism
Biguanides / chemistry,  metabolism*
Binding Sites
Cations
Chemical Precipitation
DNA / chemistry,  genetics,  metabolism*
Escherichia coli / genetics
Fluorescence Polarization
Kinetics
RNA, Transfer / genetics,  metabolism*
Titrimetry / methods
Chemical
Reg. No./Substance:
0/Anti-Infective Agents; 0/Biguanides; 0/Cations; 28757-47-3/polyhexamethylene biguanide; 9007-49-2/DNA; 9014-25-9/RNA, Transfer

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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