Document Detail


Construction of substituted cyclohexanones by reductive cyclization of 7-oxo-2,8-alkadienyl esters.
MedLine Citation:
PMID:  11772095     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Abstract/OtherAbstract:
[reaction: see text] Cyclization of 7-oxo-2,8-alkadienyl esters upon reaction with triphenylphosphinecopper hydride hexamer stereoselectively yields substituted cyclohexanones having a cis relationship of carbon side chains at C2 and C3. This cyclohexanone construction is particularly useful for preparing 4-alkoxy- or 4-siloxy-2,3-disubstituted cyclohexanones, in which instance stereoselection is > or = 20:1.
Authors:
Theodore M Kamenecka; Larry E Overman; Sylvie K Ly Sakata
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Organic letters     Volume:  4     ISSN:  1523-7060     ISO Abbreviation:  Org. Lett.     Publication Date:  2002 Jan 
Date Detail:
Created Date:  2002-01-04     Completed Date:  2002-02-19     Revised Date:  2003-10-31    
Medline Journal Info:
Nlm Unique ID:  100890393     Medline TA:  Org Lett     Country:  United States    
Other Details:
Languages:  eng     Pagination:  79-82     Citation Subset:  -    
Affiliation:
Department of Chemistry, University of California, Irvine, 516 Rowland Hall, Irvine, California 92697-2025, USA.
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