| Colloidal cluster crystallization dynamics. | |
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MedLine Citation:
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PMID: 23039607 Owner: NLM Status: In-Data-Review |
Abstract/OtherAbstract:
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The crystallization dynamics of a colloidal cluster is modeled using a low-dimensional Smoluchowski equation. Diffusion mapping shows that two order parameters are required to describe the dynamics. Using order parameters as metrics for condensation and crystallinity, free energy, and diffusivity landscapes are extracted from Brownian dynamics simulations using Bayesian inference. Free energy landscapes are validated against Monte Carlo simulations, and mean first-passage times are validated against dynamic simulations. The resulting model enables a low-dimensional description of colloidal crystallization dynamics. |
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Authors:
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Daniel J Beltran-Villegas; Ray M Sehgal; Dimitrios Maroudas; David M Ford; Michael A Bevan |
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Publication Detail:
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Type: Journal Article |
Journal Detail:
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Title: The Journal of chemical physics Volume: 137 ISSN: 1089-7690 ISO Abbreviation: J Chem Phys Publication Date: 2012 Oct |
Date Detail:
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Created Date: 2012-10-08 Completed Date: - Revised Date: - |
Medline Journal Info:
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Nlm Unique ID: 0375360 Medline TA: J Chem Phys Country: United States |
Other Details:
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Languages: eng Pagination: 134901 Citation Subset: IM |
Affiliation:
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Chemical and Biomolecular Engineering, Johns Hopkins University, Baltimore, Maryland 21218 USA. |
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From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine
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