Document Detail


Characterization of brightness and stoichiometry of bright particles by flow-fluorescence fluctuation spectroscopy.
MedLine Citation:
PMID:  21044607     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Characterization of bright particles at low concentrations by fluorescence fluctuation spectroscopy (FFS) is challenging, because the event rate of particle detection is low and fluorescence background contributes significantly to the measured signal. It is straightforward to increase the event rate by flow, but the high background continues to be problematic for fluorescence correlation spectroscopy. Here, we characterize the use of photon-counting histogram analysis in the presence of flow. We demonstrate that a photon-counting histogram efficiently separates the particle signal from the background and faithfully determines the brightness and concentration of particles independent of flow speed, as long as undersampling is avoided. Brightness provides a measure of the number of fluorescently labeled proteins within a complex and has been used to determine stoichiometry of protein complexes in vivo and in vitro. We apply flow-FFS to determine the stoichiometry of the group specific antigen protein within viral-like particles of the human immunodeficiency virus type-1 from the brightness. Our results demonstrate that flow-FFS is a sensitive method for the characterization of complex macromolecular particles at low concentrations.
Authors:
Jolene Johnson; Yan Chen; Joachim D Mueller
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Publication Detail:
Type:  Journal Article; Research Support, N.I.H., Extramural    
Journal Detail:
Title:  Biophysical journal     Volume:  99     ISSN:  1542-0086     ISO Abbreviation:  Biophys. J.     Publication Date:  2010 Nov 
Date Detail:
Created Date:  2010-11-03     Completed Date:  2011-01-28     Revised Date:  2011-11-03    
Medline Journal Info:
Nlm Unique ID:  0370626     Medline TA:  Biophys J     Country:  United States    
Other Details:
Languages:  eng     Pagination:  3084-92     Citation Subset:  IM    
Copyright Information:
Copyright © 2010 Biophysical Society. Published by Elsevier Inc. All rights reserved.
Affiliation:
School of Physics and Astronomy, University of Minnesota, Minneapolis, Minnesota, USA.
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MeSH Terms
Descriptor/Qualifier:
Biophysical Phenomena
Fluorescent Dyes
HIV Antigens / chemistry
HIV-1 / chemistry
Humans
Macromolecular Substances / chemistry
Microspheres
Particle Size
Proteins / chemistry*
Spectrometry, Fluorescence / methods*
Virion / chemistry
gag Gene Products, Human Immunodeficiency Virus / chemistry
Grant Support
ID/Acronym/Agency:
GM64589/GM/NIGMS NIH HHS; R01 GM064589-10/GM/NIGMS NIH HHS
Chemical
Reg. No./Substance:
0/Fluorescent Dyes; 0/HIV Antigens; 0/Macromolecular Substances; 0/Proteins; 0/gag Gene Products, Human Immunodeficiency Virus

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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