Document Detail


Bis-morpholine-substituted perylene bisimides: impact of isomeric arrangement on electrochemical and spectroelectrochemical properties.
MedLine Citation:
PMID:  18855454     Owner:  NLM     Status:  PubMed-not-MEDLINE    
Abstract/OtherAbstract:
The synthesis and separation of the 1,6- and 1,7- isomers of N,N'-bis(n-butyl)dimorpholino-3,4:9,10-perylenetetracarboxylic acid bisimide are reported. Investigations of the electrochemical and spectroscopic, in particular, spectroelectrochemical, properties of the two isomers reveal a sequence of electrochemically and chemically reversible redox processes for both isomers. Importantly, the 1,7-isomer of N,N'-bis(n-butyl)dimorpholino-3,4:9,10-perylenetetracarboxylic acid bisimide was observed to undergo a two-electron oxidation process, which contrasts with the behavior of both the corresponding 1,6-isomer and other related amino-substituted perylene bis-imide species.
Authors:
Gudrun Goretzki; E Stephen Davies; Stephen P Argent; Wassim Z Alsindi; Alexander J Blake; John E Warren; Jonathan McMaster; Neil R Champness
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Publication Detail:
Type:  Journal Article     Date:  2008-10-15
Journal Detail:
Title:  The Journal of organic chemistry     Volume:  73     ISSN:  1520-6904     ISO Abbreviation:  J. Org. Chem.     Publication Date:  2008 Nov 
Date Detail:
Created Date:  2008-11-14     Completed Date:  2009-01-09     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  2985193R     Medline TA:  J Org Chem     Country:  United States    
Other Details:
Languages:  eng     Pagination:  8808-14     Citation Subset:  -    
Affiliation:
School of Chemistry, University of Nottingham, University Park, Nottingham NG7 2RD, UK.
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