Document Detail


Application of 15N nuclear magnetic resonance spectroscopy to the determination of the stability of aryl nitrogen mustards.
MedLine Citation:
PMID:  7783158     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
An excellent correlation has been shown to exist between the 15N NMR chemical shifts of a series of aryl nitrogen mustards and the Hammett constant, sigma, which is much improved by the use of sigma-. These chemical shifts also correlate well with the hydrolysis rates of the compounds in 50% aqueous acetone at 66 degrees C and their alkylation of 4-(4'-nitrobenzyl)pyridine under similar conditions. Thus 15N NMR is a straightforward and material-conserving method for estimating the relative stabilities of aryl nitrogen mustards.
Authors:
D E Wilman; B D Palmer; W A Denny
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Publication Detail:
Type:  Journal Article; Research Support, Non-U.S. Gov't    
Journal Detail:
Title:  Journal of medicinal chemistry     Volume:  38     ISSN:  0022-2623     ISO Abbreviation:  J. Med. Chem.     Publication Date:  1995 Jun 
Date Detail:
Created Date:  1995-07-14     Completed Date:  1995-07-14     Revised Date:  2006-11-15    
Medline Journal Info:
Nlm Unique ID:  9716531     Medline TA:  J Med Chem     Country:  UNITED STATES    
Other Details:
Languages:  eng     Pagination:  2256-8     Citation Subset:  IM    
Affiliation:
Cancer Research Campaign Centre for Cancer Therapeutics, Institute of Cancer Research, Sutton, Surrey, U.K.
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MeSH Terms
Descriptor/Qualifier:
Drug Stability
Hydrolysis
Kinetics
Magnetic Resonance Spectroscopy
Nitrogen Isotopes
Nitrogen Mustard Compounds / chemistry*
Chemical
Reg. No./Substance:
0/Nitrogen Isotopes; 0/Nitrogen Mustard Compounds

From MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine


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