Document Detail


Allylcopper intermediates with N-heterocyclic carbene ligands: synthesis, structure, and catalysis.
MedLine Citation:
PMID:  20000669     Owner:  NLM     Status:  MEDLINE    
Abstract/OtherAbstract:
Allylcopper intermediates with N-heterocyclic carbene ligands are synthesized by transmetalation of allylsiloxane reagents, and the crystal structures of allylcopper compounds are reported. The allylcopper transmetalation is utilized for catalytic aldehyde allylation, which is found to be facilitated by a trifluorosilane co-catalyst.
Authors:
Vincenzo Russo; Jessica R Herron; Zachary T Ball
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Publication Detail:
Type:  Journal Article    
Journal Detail:
Title:  Organic letters     Volume:  12     ISSN:  1523-7052     ISO Abbreviation:  Org. Lett.     Publication Date:  2010 Jan 
Date Detail:
Created Date:  2010-01-11     Completed Date:  2010-03-08     Revised Date:  -    
Medline Journal Info:
Nlm Unique ID:  100890393     Medline TA:  Org Lett     Country:  United States    
Other Details:
Languages:  eng     Pagination:  220-3     Citation Subset:  IM    
Affiliation:
Department of Chemistry, Rice University, Houston, Texas 77005, USA.
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MeSH Terms
Descriptor/Qualifier:
Aldehydes / chemistry
Catalysis
Copper / chemistry*
Crystallography, X-Ray
Heterocyclic Compounds / chemical synthesis,  chemistry*
Ligands
Methane / analogs & derivatives*,  chemical synthesis,  chemistry
Models, Molecular
Molecular Structure
Organometallic Compounds / chemical synthesis,  chemistry*
Chemical
Reg. No./Substance:
0/Aldehydes; 0/Heterocyclic Compounds; 0/Ligands; 0/Organometallic Compounds; 2465-56-7/carbene; 74-82-8/Methane; 7440-50-8/Copper

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